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Nano@Tech Spring 2022 Series | Enhancing Converse Magnetoelectric Coupling through Strain Engineering in Artificial Multiferroic Heterostructures

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Abstract: Magnetoelectricity presents a unique opportunity to control the magnetic response of a material with an applied electric field or vice versa. Unfortunately only a few materials exhibit controllable magnetoelectric coupling (ME) within a single phase, and even then, the response is typically small and below room temperature. One route to enhance ME coupling is to create a composite between a ferroelectric and ferromagnetic material. This type of ME coupling can be mediated in multiple ways, but the current most successful method is through strain transfer across an interface. These artificial multiferroic heterostructures can exhibit ME coupling up to six orders of magnitude larger than within a single material. Still further improvement must be made before ultra-low power memory, logic, magnetic sensors, and wide spectrum antennas can be realized.  In this talk I will describe how ME coupling can be enhanced by simultaneously exploiting multiple strain engineering approaches. This work is conducted on heterostructures composed of Fe0.5Co0.5/Ag multilayers on (011) Pb(In1/2N1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 piezoelectric crystal substrates. When grown and measured under strain these heterostructures exhibit an effective converse magnetoelectric coefficient on order of 10-5 s/m: the highest directly measured, non-resonant value to-date. Additionally, this response occurred at room temperature and at low electric fields (< 2 kV/cm). This large effect is enabled by the magnetization reorientation caused by changing the magnetic anisotropy with strain and using multilayered magnetic materials to minimize the internal stress from deposition. This work highlights how multicomponent strain engineering enables enhanced magnetoelectric coupling in heterostructures and provides an approach to realize new energy efficient magnetoelectric applications.

Bio: Lauren Garten started as an assistant professor in Materials Science and Engineering at Georgia Tech in 2021. Prior to that she was a staff scientist at the U.S. Naval Research Lab (NRL) working on the growth and characterization of novel piezoelectric and artificial multiferroic heterostructures for sensors and electronics. Her work at NRL was supported by the Jerome and Isabella Karle Distinguished Fellowship and a National Research Council Associateship. Prior to this, she was a staff scientist in ferroelectric metrology development at Sandia National Laboratory and a post-doc at the National Renewable Energy Laboratory (NREL) where she worked on the processing and characterization of metastable photovoltaic materials. She received her Ph.D. in material science from the Pennsylvania State University on the development of piezoelectric and ferroelectric materials for tunable dielectrics, and her bachelor’s degree is in ceramic engineering from the Missouri University of Science and Technology. She has won the AFOSR Young Investigator Award, the DOE-BES Postdoctoral Research Award, the Outstanding Mentor Award from NREL, and the CalTech Young Investigator Lectureship. Her work focuses on the development of multifunctional multiferroics for energy and electronic applications, particularly at the nexus between ferroelectricity, magnetism, and photovoltaics.

Watch a live-stream of the seminar at https://tinyurl.com/NanoTechLive

Status

  • Workflow Status:Published
  • Created By:Christa Ernst
  • Created:01/06/2022
  • Modified By:Laurie Haigh
  • Modified:02/21/2022